Institute of Coal Chemistry,Chinese Academy of Sciences
Taoyuan 27th South Road,Taiyuan, 030001,China
Telephone:0351-4040420
Email:zhangbin2009@sxicc.ac.cn
https://publons.com/researcher/1578389/bin-zhang/publications/
1. Education
2008.9–2013.7 Ph.D. Chemical Engineering and Technology, Chinese Academy of Sciences, China
2004.9–2008.7 B.S. Applied Chemistry, Shaanxi Normal University, China
2. Employment
2024.04~now Professor, Institute of Coal Chemistry, Chinese Academy of Sciences, China
2017.9~2024.04 Associate Professor, Institute of Coal Chemistry, Chinese Academy of Sciences, China
2013.9–2017.09 Research Assistant, Institute of Coal Chemistry, Chinese Academy of Sciences, China
3. Research field
1) Atomic layer deposition and atomic layer etching technology
2) Dynamic catalysis
3) High-value fuel and chemical synthesis
一、学习经历
2008.9—2013.7: 中国科学院山西煤炭化学研究所,中国科学院大学,获工学博士学位,导师: 朱玉雷 研究员
2004.9—2008.7: 陕西师范大学,化学与材料科学学院,应用化学,理学学士
二、工作经历
2013.7—至今: 中国科学院山西煤炭化学研究所,研究员,副研究员,中国科学院青年促进会会员,中国科学院青年促进会优秀会员
三、研究方向
1) 原子层沉积和原子层刻蚀
2) 动态催化
3) 高值油品和化学品合成
四、主持或参与科研项目
1. 国家自然科学基金面上项目(2项),主持
2. 国家自然科学基金青年科学基金,主持
3. 中国科学院青年创新促进会会员,主持
4. 山西省优秀青年基金,主持
5. 煤转化国家重点实验室"青年人才培养计划",主持
6. 中国科学院低碳转化科学与工程重点实验室开放课题,主持
7. 煤转化国家重点实验室自主课题,主持
8. 国家重点研发计划变革性技术关键科学问题重点专项,参加
9. 壳牌前瞻科技研究项目,参加
10. 国家自然科学基金-中国科学院大科学装置联合基金重点项目,参加
11. 国家重点研发计划“可再生能源与氢能技术”重点专项,参加
12. 国家重点基础研究发展计划(973计划),参加
五. 发表论文列表 (Publication)
2024
63. Zhuo Li , Fanchun Meng, Xinchun Yang, Yuntao Qi, Yong Qin*, and Bin Zhang*. The Role of Mo Single Atoms and Clusters in Enhancing Pt Catalyst for Benzene Hydrogenation: Distinguishing Between Benzene Spillover and Electronic Effect', ACS Catalysis, 2024, 14, 5016-26.
62. Wen Liu, Runrun Shao, Lingyun Guo, Jianliang Man, Chengwu Zhang, Lihong Li, Haojiang Wang, Bin Wang, Lixia Guo,Sufang Ma, Bin Zhang, *Haipeng Diao, * Yong Qin, * Lili Yan *. Precise Design of TiO2@CoOx Heterostructure via Atomic Layer Deposition for Synergistic Sono-Chemodynamic Oncotherapy, Advanced Science, 2024, 2304046.
61. Huimin Yang, Xinchun Yang, Fanchun Meng, Shufang Zhang, Shichao Zhao, * Bin Zhang, * Yong Qin . Critical removal of surface carbonates on γ-Al2O3 to enhance nucleation of Pt atomic layer deposition. Journal of Catalysis, 2024, 431, 115364.
60. Xue, Lei; Luo, Gen; Yang, Xin-chun; Qin, Yong; Zhang, Bin*. Vapor-phase methods for synthesizing metal-organic framework thin films. The Innovation Materials, 2024, 100047
59. Liang, Haojie; Zhang, Bin*; Hong, Mei; Yang, Xinchun; Zhu, Ling; Liu, Xingchen*; Qi, Yuntao; Zhao, Shichao; Wang, Guofu; van Bavel, Alexander P.; Wen, Xiaodong; Qin, Yong*. Operando Mobile Catalysis for Reverse Water Gas Shift Reaction. Angewandte Chemie International Edition, 2024, e202318747.
58. Xin Huang, Haitao Li,* Bin Zhang, Yin Zhang, Hao Wang, Lijun Ban, Yixuan Xu, Yongxiang Zhao*. Dependence of copper(i) stability on long-range electromagnetic effects of Au under reducing atmospheres: the size effect of Au cores. Nanoscale, 2024, 16(4): 1971-1982.
57. Zemin, An, , NanMa, Yuanjie Xu, Hua Yang, Huibo Zhao,; Lizhi Wu,; Li Tan, Chao Zou, Fanchun Meng, Bin Zhang, Xiuyun Wang,, Yu Tang*. Shape dependency of CO2 hydrogenation on ceria supported singly dispersed Ru catalysts. Journal of Catalysis, 2024, 429: 115245.
2023
56. Fanchun Meng, Xinchun Yang, Shichao Zhao, Zhuo Li, Yuntao Qi, Huimin Yang, Yong Qin, Bin Zhang*. Tailoring the Brønsted acidity of Ti-OH species by regulating Pt-TiO2 interaction. ChemSusChem 2023, n/a (n/a), e202301410.
55. Liming Zhai, Bin Zhang*, Haitao Li, Min Jiang, Xinchun Yang, Zhuo Li, Shichao Zhao, Yong Qin*, ChemCatChem 2023, 15, e202300887.
54. Fanchun Meng, Xinchun Yang, Shichao Zhao, Zhuo Li, Guikai Zhang, Yuntao Qi, Shengqi Chu, Guofu Wang, Jing Zhang, Yong Qin*, Bin Zhang*. Shifting reaction path for levulinic acid aqueous-phase hydrogenation by Pt-TiO2 metal-support interaction. Applied Catalysis B: Environmental, 2023, 324, 122236.
2022
53. Zhe Wang, Bin Zhang*, Shuai Yang, Xinchun Yang, Fanchun Meng, Liming Zhai, Zhuo Li, Shichao Zhao, Guojie Zhang, Yong Qin. Dual Pd2+ and Pd0 sites on CeO2 for benzyl alcohol selective oxidation. Journal of Catalysis, 2022, 414, 385-393
52. Xinchun Yang, Caihong Xing, Bin Zhang*, Xingchen Liu*, Haojie Liang, Gen Luo, Guikai Zhang, Zhuo Li, Shichao Zhao, Jing Zhang, Guofu Wang, and Yong Qin*, Direct Bonding of CpCo- Fragments on Pt Nanoparticles and their Electronic Effect for Alkyne Semihydrogenation, ACS Catal., 2022, 12, 10849-10856.
51. Shufang Zhang, Bin Zhang*, Zhimin Li, Xinchun Yang, Fanchun Meng, Haojie Liang, Yu Lei, Huibin Wu, Jing Zhang, Gao Li*, Yong Qin*, Surface isolation of single metal complexes or clusters by a coating sieving layer via atomic layer deposition, Cell Reports Physical Science, 2022, 3, 100787
50. Haojie Liang, Bin Zhang*, Peng Gao, Xiaohu Yu*, Xingchen Liu, Xinchun Yang, Huibin Wu, Liming Zhai, Shichao Zhao, Guofu Wang, Alexander P.van Bavel, YongQin*, Strong Co-O-Si bonded ultra-stable single-atom Co/SBA-15 catalyst for selective hydrogenation of CO2 to CO, Chem Catalysis, 2022, 2 (3), 610-621.
49. Huibin Wu, Xinchun Yang, Shichao Zhao, Liming Zhai, Guofu Wang, Bin Zhang*, Yong Qin, Encapsulation of Atomically Dispersed Pt Clusters in Porous TiO2 for Semi-Hydrogenation of Phenylacetylene. Chem. Commun., 2022, 58, 1191.
2021
48. F. Wang, J.D. Harindintwali, Z. Yuan, M. Wang, F. Wang, S. Li, Z. Yin, L. Huang, Y. Fu, L. Li, S.X. Chang, L. Zhang, J. Rinklebe, Z. Yuan, Q. Zhu, L. Xiang, D.C.W. Tsang, L. Xu, X. Jiang, J. Liu, N. Wei, M. Kästner, Y. Zou, Y.S. Ok, J. Shen, D. Peng, W. Zhang, D. Barcelo, Y. Zhou, Z. Bai, B. Li, B. Zhang, K. Wei, H. Cao, Z. Tan, L.-b. Zhao, X. He, J. Zheng, N. Bolan, X. Liu, C. Huang, S. Dietmann, M. Luo, N. Sun, J. Gong, Y. Gong, F. Brahushi, T. Zhang, C. Xiao, X. Li, W. Chen, N. Jiao, J. Lehmann, Y.-G. Zhu, H. Jin, A. Schaeffer, J.M. Tiedje, J.M. Chen, Technologies and perspectives for achieving carbon neutrality, The Innovation, 2021, 100180
47. Y. Xu, Q. Wang, Z. An, F. Wang, L. Zhang, Y. Wu, F. Dong, C.-W. Qiu, X. Liu, J. Qiu, K. Hua, W. Su, H. Xu, Y. Han, X. Cao, E. Liu, C. Fu, Z. Yin, M. Liu, R. Roepman, S. Dietmann, M. Virta, F. Kengara, C. Huang, Z. Zhang, L. Zhang, T. Zhao, J. Dai, J. Yang, L. Lan, M. Luo, T. Huang, Z. Liu, S. Qian, T. An, X. Liu, B. Zhang, X. He, S. Cong, X. Liu, W. Zhang, F. Wang, C. Lu, Z. Cai, J.P. Lewis, J.M. Tiedje, J. Zhang, Artificial Intelligence: A Powerful Paradigm for Scientific Research, The Innovation, 2021, 100179
46. Gen Luo, Bin Zhang*, Xin-chun Yang, Hui-bin Wu, Fan-chun Meng, Li-ming Zhai, Yong Qin, Synthesis of ZIF-8-coated Pt/SiO2 by vapor deposition for alkyne semi-hydrogenation, Journal of Fuel Chemistry and Technology, 2021, 49(9): 1316-1325(Cover paper).
45. Liming Zhai, Bin Zhang*, Haojie Liang, Huibin Wu, Xinchun Yang, Gen Luo, Shichao Zhao & Yong Qin, The selective deposition of Fe species inside ZSM-5 for the oxidation of cyclohexane to cyclohexanone, Science China Chemistry, 2021, 64, 1088–1095
44. Shichao Zhao, Jie Yang, Feifei Duan, Baiyan Zhang, Yequn Liu, Bin Zhang, Chaoqiu Chen, Yong Qin*, Rational construction of porous N-doped Fe2O3 films on porous graphene foams by molecular layer deposition for tunable microwaveabsorption, J. Colloid Interface Sci., 2021, 598, 45-55
2020
43. Huibin Wu, Bin Zhang*, Haojie Liang, Liming Zhai, Guofu Wang, Yong Qin*, Distance Effect of Ni-Pt Dual Sites for Active Hydrogen Transfer in Tandem Reaction, The Innovation, 2020, 1(2), 100029.
42. 翟黎明,张斌*,梁浩杰,武慧斌,覃勇*,原子层沉积制备FeO_x/ZSM-5催化剂及其甲烷液相氧化性能,天然气化工, 2020, 45(253), 7-12.
41. Huibin Ge, Bin Zhang*, Haojie Liang, Mingwei Zhang, Kegong Fang, Yao Chen,Yong Qin*, Photocatalytic Conversion of CO2 into Light Olefins over TiO2 Nanotube confined Cu Clusters with high ratio of Cu+, Appl. Catal. B: Environ., 2020, 263, 118133.
40. Zhifeng Jiao, Ya-Ming Tian, Bin Zhang*, Cai-Hong Hao, Yan Qiao, Ying-Xiong Wang, Yong Qin, Udo Radius, Holger Braunschweig, Todd B.Marder, Xiao-Ning Guo*, Xiang-Yun Guo, High Photocatalytic Activity of a NiO Nanodot-decorated Pd/SiC Catalyst for the Suzuki-Miyaura Cross-coupling of Aryl Bromides and Chlorides in Air under Visible Light, Journal of Catalysis, 2020, 389, 517-524.
39. Lili Yan, Min Zhang, Shichao Zhao, Tijian Sun, Bin Zhang, Maosheng Cao*, YongQin*, Wire-in-tube ZnO@carbon by molecular layer deposition: Accurately tunable electromagnetic parameters and remarkable microwave absorption, Chem. Eng. J., 2020, 382, 122860.
2019
38. Zheng Lu, Xiaoyang Liu, Bin Zhang, Zhuoran Gan, Siwen Tang, Lu Ma, Tianping Wu, George J. Nelson, Yong Qin, C. Heath Turner, Yu Lei*, Structure and Reactivity of Single Site Ti Catalysts for Propylene Epoxidation, J.Catal., 2019, 377, 419-428.
37. Zhifeng Jiao, Jixiao Zhao, Xiaoning Guo*, Xili Tong, Bin Zhang, Guoqiang Jin, Yong Qin, Xiangyun Guo*, Turning the product selectivity of nitrile hydrogenation from primary to secondary amines by precise modification of Pd/SiC catalysts using NiO nanodots, Catal. Sci. Technol., 2019, 121, 48-52.
36. M.qahtani*, S. Ben-Jabar, M. Ebaid, S. Sathasivam, P. Jurczak, X. Xia, A. Alromaeh, C. Blackman, Y. Qin, B. Zhang, B. S. Ooi, H. Liu, I. P. Parkin, and J. Wu., Gallium Phosphide photoanode coated with TiO2and CoOx for stable photoelectrochemical water oxidation. Optics Express, 2019, 27(8), A364-A371.
35. Dan Xu, Shuyuan Wang, Baoshan Wu*, Bin Zhang, Yong Qin*, Chunfang Huo, Lihua Huang, Xiaodong Wen, Yong Yang, Yongwang Li*, Highly Dispersed Single-Atom Pt and Pt Clusters in the Fe-Modified KL Zeolite with Enhanced Selectivity for n-Heptane Aromatization, ACS Appl. Mater. Interfaces, 2019, 11(33), 29858-29867.
34. 陈长胜, 张斌, 覃勇*, 原子层沉积技术选择性修饰Mo/HZSM-5对甲烷无氧芳构化反应的影响,现代化工 2019, 39(12), 191-194.
2018
33. B. Zhang, Y. Qin*, Interface tailoring of heterogeneous catalysts by atomic layer deposition, ACS Catal. 2018, 10064-10081. (Invited review)
32. S. Zhang, B. Zhang*, H.J. Liang, Y. Liu, Y. Qiao, Y. Qin*. Encapsulation of Homogeneous Catalysts in Mesoporou`s Materials Using Diffusion-Limited Atomic Layer Deposition, Angew. Chem. Int. Ed. 2018, 57 (4), 1091-1095.
31. H. Yang, B.Y. Zhang, B. Zhang, Z. Gao, Y.Qin*. N-doped carbon modified Pt/CNTs synthesized by atomic layer deposition with enhanced activity and stability for methanol electrooxidation. Chinese J. Catal. 2018, 39 (6), 1038-1043.
30. F. Zhang, B. Zhang, X. Wang, L. Huang*, D. Ji, S. Du, L. Ma, S. Lin. Synthesis of Tetrahydropyran from Tetrahydrofurfuryl Alcohol over Cu–ZnO/Al2O3 under a Gaseous-Phase Condition. Catalysts 2018, 8 (3), 105.
29. X. Song, H. Zhang, Y. Yang, B. Zhang, M. Zuo, X. Cao, J. Sun, C. Lin, X.P. Li*, Z. Jiang*. Bifunctional Nitrogen and Cobalt Codoped Hollow Carbon for Electrochemical Syngas Production. Adv. Sci. 2018, 1800177.
28. D. Xu, S. Wang, B. Wu, C. Huo, Y. Qin, B. Zhang, J. Yin, L. Huang, X. Wen, Y. Yang, Y. Li, Tailoring Pt locations in KL zeolite by improved atomic layer deposition for excellent performance in n-heptane aromatization. J. Catal. 2018, 365, 163-173.
27. X.C. Niu, D.P. Cao*, B. Zhang, X.C. Liu, X.D. Wen, Y, Qin, J.G. Wang, Surface structure of zinc ferrite (311)-A density functional theory study (铁酸锌(311)表面结构的密度泛函理论研究). J. Fuel Chem. Tech. (燃料化学学报) 2018, 46(8), 985-991.
26. Alqahtani M., Sathasivam S.,Alhassan A., Cui F., BenJaber S., Blackman C., Zhang B., Qin Y., Parkin I. P., Nakamura S., Liu H., Wu J., InGaN/GaN Multiple Quantum Well Photoanode Modified with Cobalt Oxide for Water Oxidation. ACS Appl. Energy Materials 2018, 1(11), 6417-6424.
2017
25. Jiquan Liu, Pedro B. Groszewicz, Qingbo Wen, Aany Sofia Lilly Thankamony, Bin Zhang, Ulrike Kunz, Grit Sauer, Yeping Xu, Torsten Gutmann*, Gerd Buntkowsky*, Revealing Structure Reactivity Relationships in Heterogenized Dirhodium Catalysts by Solid-State NMRTechniques, Journal of Physical Chemistry C, 2017, 121(32), 17409-17416.
24. H.J. Liang, B. Zhang*, H.B. Ge, X.M. Gu, S.F. Zhang, and Y. Qin*. Porous TiO2/Pt/TiO2 sandwich catalyst for highly selective semi-hydrogenation of alkyne to olefin. ACS Catal. 2017, 7, 6567-6572.
23. X.M. Gu, B. Zhang*, H.J. Liang, H.B. Ge, H.M. Yang, and Y. Qin*. Pt/HZSM-5 catalyst synthesized by atomic layer deposition for aqueous-phase hydrogenation of levulinic acid to valeric acid. J. Fuel Chem. Tech. 2017, 45(6), 714-722.
22. Y. Zhu, X. Kong, J. Yin, R. You, B. Zhang, H. Zheng, X. Wen*, Y. Zhu*, Y. W. Li. Covalent-bonding to irreducible SiO2 leads to high-loading and atomically dispersed metal catalysts. J. Catal. 2017, 353, 315-324.
21. D. Xu, B. Wu*, P. Ren, S. Wang, C. Huo, B. Zhang, W. Guo, L. Huang, X. Wen, Y. Qin, Y. Yang*, Y. Li*, Controllable deposition of Pt nanoparticles into KL zeolite by atomic layer deposition for highly efficient reforming of n-heptane to aromatics. Catal. Sci. Tech. 2017, 7, 1342-1350.
20. L. Yan, X. Wang, S. Zhao, Y. Li, Z. Gao, B. Zhang, M. Cao, Y. Qin*. Highly Efficient Microwave Absorption of Magnetic Nanospindle-Conductive Polymer Hybrids by Molecular Layer Deposition. ACS Appl. Mater. Interfaces 2017, 9,11116-11125.
19. L. Yan, J. Liu, S. Zhao, B. Zhang, Z. Gao, H. Ge, Y. Chen, M. Cao, Y. Qin*, Coaxial multi-interface hollow Ni-Al2O3-ZnO nanowires tailored by atomic layer deposition for selective frequency absorptions. Nano Research 2017, 10(5), 1595-1607.
2016
18. H. B. Ge, B. Zhang*, X. Gu, H. J. Liang, H. M. Yang, Z. Gao, J. G. Wang, and Y. Qin*. A tandem catalyst with multiple metal-oxide interfaces produced by atomic layer deposition. Angew. Chem. Int. Ed. 2016, 55, 7081-7085. (Very important paper,物理化学学报、ChemistryViews等推送报道)
17. B. Zhang, X. W. Guo, H. J. Liang, H. B. Ge, X. M. Gu, S. Chen, H. M. Yang, Y. Qin*. Tailoring Pt-Fe2O3 interfaces for selective reductive coupling reaction to synthesize imine. ACS Catal. 2016, 6, 6560-6566.
16. X.M. Xiang, B. Zhang, G. Q. Ding, J.L. Cui, H. Y. Zheng,Y. L. Zhu*. The effect of Mg(OH)2 on furfural oxidation with H2O2. Catal. Commun. 2016, 86, 41-45.
15. M.H. Wang, Z. Gao*, B. Zhang, H. M. Yang, Y. Qiao, S. Chen, H.B. Ge, J.K. Zhang, Y. Qin*. Ultrathin coating of confined Pt nanocatalysts by atomic layer deposition for enhanced catalytic performance in hydrogenation reactions. Chem. Eur. J. 2016, 22, 8438-8443. (Cover paper)
14. Y. Chen, Z. Gao, B. Zhang, S.C. Zhao, Yong Qin*, Graphene coated with controllable n-doped carbon layer by molecular layer deposition as electrode materials for super capacitors. J. Power Sources 2016, 315,254-260.
13. J.K. Zhang, C.Q Chen*, W.J. Yan, F.F. Duan, B. Zhang, Z. Gao, Y. Qin*. Ni nanoparticles supported on CNTs with excellent activity produced by atomic layer deposition for hydrogen generation from hydrolysis of ammonia borane. Catal. Sci. Technol. 2016, 6, 2112 - 2119.
12. S.C. Zhao, Z. Gao, C.Q. Chen, G.Z. Wang, B. Zhang, Y. Chen, J. Zhang, X. Li, Y. Qin*. Alternate nonmagnetic and magnetic multilayer nanofilms deposited on carbon nanocoils by atomic layer deposition to tune microwave absorption property. Carbon 2016, 98, 196-203.
2015
11. B. Zhang, Y. Chen, J.W. Li, E. Pippel, H. M. Yang, Z. Gao, and Y. Qin*. High efficiency Cu-ZnO hydrogenation catalyst: the tailoring of Cu-ZnO interface sites by molecular layer deposition. ACS Catal. 2015, 5, 5567–5573.
10. J.W. Li, B. Zhang, Y. Chen, J. K. Zhang, H. M. Yang, J. W. Zhang, X. L. Lu, G. C. Li*, and Y. Qin*. Styrene hydrogenation performance of Pt nanoparticles with controlled size prepared by atomic layer deposition. Catal. Sci. Technol. 2015, 5, 4218-4223.
9. Y. Chen, B. Zhang, Z. Gao, C.C. Chen, S.C. Zhao, Y. Qin*. Functionalization of multiwalled carbon nanotubes with uniform polyurea coatings by molecular layer deposition. Carbon 2015, 82, 470-478.
8. C.C. Lv, Z.B Chen, Z.Z. Chen, B. Zhang, Y. Qin, Z.P. Huang,* C. Zhang*. Silicon nanowires loaded with iron phosphide for effective solar-driven hydrogen production. J. Mater. Chem. A 2015, 3(34), 17669-17675.
7. Z. Gao, M. Dong, G.Z. Wang, P. Sheng, Z.W. Wu, H.M. Yang, B. Zhang, G.F. Wang, J.G. Wang, Y. Qin*. Multiply confined nickel nanocatalysts produced by atomic layer deposition for hydrogenation reactions. Angew. Chem. Int. Ed. 2015, 54(31), 9006–9010.
2014
6. B. Zhang, G. Q. Ding, H. Y. Zheng, and Y. L. Zhu*. Transesterification of dimethyl carbonate with tetrahydrofurfuryl alcohol on the K2CO3/ZrO2 catalyst—function of the surface carboxylate species. Appl. Catal. B: Env. 2014, 152–153, 226-232.
2011-2013
5. B. Zhang, Y. L. Zhu*, G. Q. Ding, H. Y. Zheng, and Y. W. Li. Selective conversion of furfuryl alcohol to 1,2-pentanediol over a Ru/MnOx catalyst in aqueous phase. Green Chem. 2012, 14, 3402-3409.
4 B. Zhang, Y. L. Zhu*, G. Q. Ding, H. Y. Zheng, and Y. W. Li. Modification of the supported Cu/SiO2 catalyst by alkaline earth metals in the selective conversion of 1,4-butanediol to γ-butyrolactone. Appl. Catal. A: Gen. 2012, 443-444, 191-201.
3. L.G. Chen, Y.L. Zhu*, H.Y. Zheng, C.H. Zhang, B. Zhang, Y.W. Li. Catalytic degradation of oxygenates in Fischer–Tropsch aqueous phase effluents to fuel gas via hydrodeoxygenation over Ru/AC catalyst. J. Chem. Tech. Bio. 2012, 87, 112-122.
2. S. Zhu, Y. Zhu, S. Hao, L. Chen, B. Zhang, Y. Li. Aqueous-phase hydrogenolysis of glycerol to 1,3-propanediol over Pt-H4SiW12O40/SiO2. Catal. Lett. 2012, 142, 267-274.
1. L.G. Chen, Y.L. Zhu*, H.Y. Zheng, C.H. Zhang, B. Zhang, Y.W. Li. Aqueous-phase hydrodeoxygenation of carboxylic acids to alcohols or alkanes over supported Recatalysts. J. Mol. Catal. A: Chem. 2011, 351, 217-227.